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LiCoO2 particles were coated with 33Li4GeS4·67Li3PS4 (mol%) solid electrolyte (SE) thin films by pulsed laser deposition (PLD). The all-solid-state cells using positive electrodes, composed of only LiCoO2 particles coated with SE thin films, were fabricated and their electrochemical performances were investigated. The cell was charged and discharged with a higher capacity of 67mAhg−1 than that using LiCoO2 particles without SE-coating. Moreover, the capacity of all-solid-state cell increased to 80mAhg−1 after enhancing the ionic conductivity of SE thin films by heat treatment at 200°C. The use of highly lithium-ion conductive thin films was effective in the formation of sufficient lithium-ion conduction paths in positive electrodes for bulk-type all-solid-state batteries. © The Electrochemical Society of Japan, All rights reserved.

Bulk-type All-solid-state Lithium Secondary Batteries Using Highly Ion-conductive Sulfide Solid Electrolyte Thin Films