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“Smartly” functionalized carbon nanotubes (CNTs) constitute an actively pursued research topic in the fields of nanomaterials and nanotechnology. The development of highly efficient and selective methodologies for dispersing CNTs in the liquid phase has not only made efficient separation and purification of CNTs possible, but also opened the doors to many fascinating material and biological applications. Very recently, the development of CNT hybrid systems with controlled stimuli-responsiveness has achieved significant breakthroughs. This chapter outlines the state of the art within this vibrant research area, and examples from the most recent literature are selected to demonstrate progress in the preparation of CNT composites, the physical properties of which can be readily switched by various external stimuli (e.g., pH, photoirradiation, solvent, temperature, etc.).

Functionalization of Carbon Nanotubes with Stimuli- Responsive Molecules and Polymers