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The phosphazenes have distinguished ancestry. The reaction between phosphorus pentachloride and ammonia was described by Rose in 1834[1], and in an editorial comment, Liebig [13] reported work carried out in conjunction with Wohler. The major reaction product was phospham and a small quantity of a stable crystalline compound containing nitrogen, phosphorus, and chlorine was obtained. Gerhardt and Laurent established that the empirical composition was NPCl2, and Gladstone and Holmes and Wichelhaus measured the vapor density and deduced the molecular formula, N3P3Cl6[2].

Theoretical Study for High Energy Density Compounds from Cyclophosphazene