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Compounds containing the P(O)(N)n(O)3-n (n = 1, 2, 3), P(O)(N)m(O)2-mX (m = 1, 2, X = C, Cl, F, S etc.) and P(O)(O)3 moieties are among the well-studied inorganic compounds [an interested reader may find many examples of compounds with the mentioned skeletons through a CSD search, [1]]. N,N,N',N',N",N"-hexamethyl phosphoric triamide (HMPA, Scheme 1) is an important polar aprotic solvent with a high-dielectric constant [2] and an excellent ligand for interaction with hard metal-cations [3].

Phosphoramidates: Molecular Packing and Hydrogen Bond Strength in Compounds Having a P(O)(N)n(O)3-n (n = 1, 2, 3) Skeleton