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The objective of this study was to estimate the source apportionment at the Pinnacles National Monument IMPROVE site in western coastal USA. The PMF was applied to identify the existing sources and apportion the mass to each source. To analyze local source impacts from various wind directions, the NPR analysis was performed using source contribution results with the wind direction values measured at the site. Also, PSCF was applied to identify the locations by point sources relative to the back trajectories. A total of 1,634 samples were collected from March 1988 to May 2004 by IMPROVE sampler and 32 chemical species were analyzed by PIXE, PESA, XRF, IC, and TOR methods. The PMF modeling identified seven sources and the average mass was apportioned to gasoline vehicle, secondary sulfate, aged sea salt, secondary nitrate, wood/field burning, diesel emission, and soil, respectively. In this study, the average mass was apportioned to gasoline vehicle (33.0%), secondary sulfate (25.7%), aged sea salt (17.8%), and secondary nitrate (10.1%). Also, this study suggests the possible role for source apportionment study of at similar areas such as wildness, national park, and coastal areas in Korea.

Source Identification and Estimation of Source Apportionment of Ambient PM2.5at Western National Park Site in USA

Source Identification and Estimation of Source Apportionment of Ambient PM_2.5at Western National Park Site in USA