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The collective excitations in water are studied based on the interactionsite\udmodel of liquids. Three collective modes, extracted from a generalized\udLangevin equation combined with the RISM theory of liquids, are identified\udas an acoustic mode and two optical modes. The drag force exerted on ions\udin water is described in terms of the response of these solvent collective\udexcitations to the perturbation of ions. The ion-size dependence of the drag\udforce, which has been a central issue in physical chemistry for long time, is\udstudied in molecular detail based on the novel approach

COLLECTIVE DENSITY FLUCTUATIONS AND DYNAMICS OF IONS IN WATER STUDIED BY THE INTERACTION-SITE MODEL OF LIQUIDS