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The heterogeneous reaction of N2O5 on mixed organic-inorganicaerosol particles was investigated using an entrained aerosol flow tubecoupled to a custom-built chemical ionization mass spectrometer. Laboratoryresults on aqueous particles confirm a strong dependence of the reactiveuptake coefficient (γ) on particle liquid water, for particle waterconcentrations below 15 M, and the molar ratio of particle water to nitrate.Measurements of γ (N2O5) on mixed chloride-nitrateparticles indicate that the presence of trace chloride can negate thesuppression of γ(N2O5) at high nitrate loadings withimplications for polluted coastal regions. These results are used toconstruct a new parameterization for γ (N2O5), that whencoupled to an aerosol thermodynamics model, can be used within regionaland/or global chemical transport models

atmospheric chemistry and physics

Toward a general parameterization of N&amp;lt;sub&amp;gt;2&amp;lt;/sub&amp;gt;O&amp;lt;sub&amp;gt;5&amp;lt;/sub&amp;gt; reactivity on aqueous particles: the competing effects of particle liquid water, nitrate and chloride