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The isotopically substituted nitrous oxide species 14N14NO, 15N14NO,14N15NO and 15N15NO were investigated byultra-violet (UV) absorption spectroscopy. High precision cross sectionswere obtained for the wavelength range 181 to 218nm at temperatures of 233and 283K. These data are used to calculate photolytic isotopicfractionation constants as a function of wavelength. The fractionationconstants were used in a three-dimensional chemical transport model in orderto simulate the actual fractionation of N2O in the stratosphere, andthe results were found to be in good agreement with field studies

atmospheric chemistry and physics

Ultra-violet absorption cross sections of isotopically substituted nitrous oxide species: &amp;lt;sup&amp;gt;14&amp;lt;/sup&amp;gt;N&amp;lt;sup&amp;gt;14&amp;lt;/sup&amp;gt;NO, &amp;lt;sup&amp;gt;15&amp;lt;/sup&amp;gt;N&amp;lt;sup&amp;gt;14&amp;lt;/sup&amp;gt;NO, &amp;lt;sup&amp;gt;14&amp;lt;/sup&amp;gt;N&amp;lt;sup&amp;gt;15&amp;lt;/sup&amp;gt;NO and &amp;lt;sup&amp;gt;15&amp;lt;/sup&amp;gt;N&amp;lt;sup&amp;gt;15&amp;lt;/sup&amp;gt;NO