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Sander et al. (2006) proposed that CaCO<sub>3</sub> precipitation can be an  important factor in triggering tropospheric ozone depletion events.  Recently, Morin et al. (2008b) presented calculations with the FREZCHEM model  and concluded that their results and interpretation cast doubt on the  validity of this hypothesis. In this joint publication, we have  re-analyzed the implications of the FREZCHEM results and show how they  can be reconciled with the proposal of Sander et al. (2006). The chemical  predictions of both approaches are consistent. Although an  interpretation solely based on the alkalinity change in the brine does  not support the conclusion of Sanderet al. (2006), we show that the  bromide/alkalinity ratio (which increases during the cooling of the  brine) can be used as an indicator of the potential for triggering  bromine explosions

atmospheric chemistry and physics

Introducing the bromide/alkalinity ratio for a follow-up discussion on &amp;quot;Precipitation of salts in freezing seawater and ozone depletion events: a status report&amp;quot;, by Morin et al., published in Atmos. Chem. Phys., 8, 7317–7324, 2008