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Various organosilicon compounds act as synthetic equivalents of unstable active chemical species, especially novel 1, 3-dipolar reagents such as azomethine ylides, thiocarbonyl ylides and related reagents, are designed and synthesized. These compounds activated by a Lewis acid or fluoride ion react with a variety of dipolarophiles and hetero-dipolarophiles in highly regio- and stereospecific mode. It has been found that this methodology can be extended to the design and preparations of tailor-made 1, 3-dipolar reagents. The highly selective synthesis of heterocycles are described.

yūki gōsei kagaku kyōkaishi/yuuki gousei kagaku kyoukaishi

Synthesis of Organosilicon Compounds as Synthetic Equivalents of Unstable Active Chemical Species and Their Applications to Highly Selective Synthesis of Heterocycles.