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Han-Gook Cho Department of Chemistry, University of Incheon, Incheon 406-772, Korea. E-mail: hgc@incheon.ac.krReceived March 2, 2014, Accepted March 18, 20142H-azirine, a less known acetonitrile isomer, is observed in matrix IR spectra from the precursor exposed toradiation from laser ablation of transition-metals. Its vibrational characteristics confirm the previous results,and those for the deuterated and

Matrix Infrared Spectra and DFT Computations of 2H-Azirine Produced from Acetonitrile by Laser-Ablation Plume Radiation