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E-mail: kimjn@chonnam.ac.krReceived January 27, 2014, Accepted February 12, 2014A practical and efficient one-pot synthesis of 1,3,5-trisubstituted pyrazoles from α,β-enones and arylhydrazinehydrochlorides has been developed. The pyrazoles were formed via a tandem formation of the correspondingpyrazolines and an acid-catalyzed aerobic oxidation process.Key Words : Pyrazoles, One-pot synthesis, Aerobic oxidation, α,β-Enones Introduction1,3,5-Trisubstituted pyrazolines are important heterocycliccompounds which can be prepared from substituted hydra-zines and α,β-enones. The oxidation of these pyrazolinesprovides the corresponding pyrazoles, which are known topossess diverse biological activities.

Facile One-Pot Synthesis of 1,3,5-Trisubstituted Pyrazoles from α,β-Enones