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process) in a high [amine] region. This contrasts to the recent report that the corresponding aminolysis of benzyl2-pyridyl carbonate 5 proceeds through a forced concerted mechanism. An intramolecular H-bondinginteraction was suggested to force the reactions of 5 to proceed through a concerted mechanism, since it couldaccelerate the rate of leaving-group expulsion (i.e., an increase in k

bulletin of the korean chemical society

Aminolysis of Benzyl 4-Pyridyl Carbonate in Acetonitrile: Effect of Modification of Leaving Group from 2-Pyridyloxide to 4-Pyridyloxide on Reactivity and Reaction Mechanism