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Six metal-free organic dyes having thiophene (1), benzene-thiophene (2), thiophene-benzene (3), thiophene-pyridine (4), thiophene-thiophene (5), and pyridine (6) linkers between 9,9-dimethylfluorenyl terminal group and α-cyano-acrylic acid anchor were synthesized. Among them, organic dye 5 showed the longest λ max value (424 nm) in UV-Vis absorption spectrum, better incident monochromatic photon-to-current conversion efficiency (IPCE), highest short circuit photocurrent density (J SC , 9.33 mA 2 /cm 2 ), and highest overall conversion efficiency (η, 3.91%).

bulletin of the korean chemical society

Synthesis of Organic Dyes with Linkers Between 9,9-Dimethylfluorenyl Terminal and α-Cyanoacrylic Acid Anchor, Effect of the Linkers on UV-Vis Absorption Spectra, and Photovoltaic Properties in Dye-Sensitized Solar Cells