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Inorganic materials such as lithium niobate have manydisadvantages such as slow response time and degradativephotorefractive effects, which limit their applications. NLOpolymers, on the other hand, are considered candidatematerials, mainly because they offer many advantages suchas mechanical endurance, light weight, chemical resistance,and good processability to form optical devices. One of thecurrent challenges is to design novel NLO polymers havingoptimized properties. In the developments of NLO polymersfor electro-optic device applications, stabilization of elec-trically induced dipole alignment is an important consider-ation; in this context two approaches to minimize therandomization have been proposed namely the use of cross-linking

Preparation of Novel T-type Polyurethanes with High Thermal Stability of Second Harmonic Generation and Their Nonlinear Optical Properties