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Much of this activity has been associatedwith the synthesis of macrocyclic ligands that exhibit highselectivity for specific metal ions. In most cases, the prepara-tion of mixed donor macrocyclic compounds requiresseveral steps and/or results in low yield. Metal directed condensation reactions involving coordi-nated polyamines and formaldehyde have been utilized forthe preparation of various types of saturated polyazamacrocyclic compounds that could not be prepared by othermethods.

Template Synthesis of Copper(II) Complexes of N3O-Donor Macrotricycles Containing N-CH2-N and N-CH2-O Linkages

Template Synthesis of Copper(II) Complexes of N₃O-Donor Macrotricycles Containing N-CH₂-N and N-CH₂-O Linkages