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Research Institute of Industrial Technology, Kyungpook National University, Taegu 702-701, KoreaDepartment of Industrial Chemistry, College of Engineering, Kyungpook National University, Taegu 702-701, KoreaReceived October 12, 2001Keywords : Aldehyde, Catalyst, Ruthenium, Reductive amination, Tertiary amine.The reductive amination of ketones and aldehydes withamines has been used as a tool for N-alkylation of amines.The process generally proceeds in two tandem steps,condensation between carbonyl compounds and amines toform an imine and reduction of the imine by a reducingagent.

An Unprecedented Ruthenium-Catalyzed Reductive Amination of Aldehydes with Tertiary Amines