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We have investigated the H/D exchange reaction between heavy water and an ionic liquid, 1-butyl-3-methyl-imidazolium tetrafluoroborate ([bmim][BF4]), throughout the whole concentration region as a function of D<sub>2</sub>O mol% at room temperature. We expected that the extent of the H/D reaction would increase linearly with increasing content of D<sub>2</sub>O, but the results show an extended N-shaped behavior having a small maximum at around 40 mol% and the reaction becomes very slow at a specific concentration around 80 mol%. We found that this non-linear concentration dependence correlates with the pD dependence of the solutions

open journal of physical chemistry

Peculiar Concentration Dependence of H/D Exchange Reaction in 1-Butyl-3-methylimidazolium Tetrafluoroborate-D&amp;lt;sub&amp;gt;2&amp;lt;/sub&amp;gt;O Mixtures