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Cyano-4,6-dimethyl-2-oxo-2H-pyridin-1-ylmethyl)benzyloxy)-4,6-dimethyl- nicotinonitrile (1) has been synthesized and characterized by 1 H and 13 C NMR. In solid state, the molecular conformation of sterically hindered compound (1) is stabilized in such a way that gauche conformation is attained by both heterocyclic rings with respect to phenyl ring via intramolecular CH-O and CH-π interactions. The weak CH-X (π, O, N) interactions manifest an interesting role in stabilizing the packing mode of compound. X-ray crystal structure of compound shows a cavity of 13 members formed via intramolecular CH-π interaction.

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Conformational tuning of molecular network stabilized via C-H….π &amp; π-π interaction in 2-[2-(3-cyano-4, 6-dimethyl-2-oxo-2H-pyridin-1-yl-methyl)-benzyloxy]-4, 6-dimethyl-nicotinonitrile