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S-Methylisothioureas, 2-N―H, -N―alkyl and -N―aryl are synthesized from the reaction of ammonia or the corresponding aromatic amines with benzothiazole dithiomethylcarboimidate. The reaction with pyrrolidine and piperazine are reported. Compounds were characterized by 1 H and 13 C NMR spectroscopy and the X-ray molecular structure of S-methy-N- benzothiazolelisothiourea derivative is reported.

S-Methyl-(-N-aryl and -N-alkyl)isothioureas derived from 2-aminobenzothiazole