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E)-3-Phenylsulfonylprop-2-enenitrile reacts with sulfur-, oxygenand carbon-based nucleophiles to yield (E)-configured β-substituted α,β-unsaturated nitriles via a regiospecific addition-elimination sequence.

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Addition of nucleophiles to (E)-3-phenylsulfonylprop-2-enenitrile: a route to β-substituted α,β-unsaturated nitriles and to acetals of cyanoacetaldehyde