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Double annelation of an imidazo[1,2-a]pyrimidine moiety was achieved in a one-pot process by reacting heteroaromatic 2-aminoesters and 2-aminonitriles with 2-(methylthio)-2-imidazoline, obtaining a number of mostly novel tetracyclic hetero-systems.

Reagents for new heteroannelation reactions part V: 2-(methylthio)-2-imidazoline