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xx 1  Introduction  1 1.1 Sources of PBTs and health impacts of ecosystem contamination on humans and wildlife  2 1.2 The role of gaseous air-water exchange in forecasting trends in ecosystem contamination  4 1.3 Dissertation overview  6 2  Gas-phase cleanup method for analysis of trace atmospheric semivolatile organic compounds by thermal desorption from diffusion denuders  9 2.1 Abstract  9 2.2 Introduction  9 2.3 Experimental  13 2.3.1  Chemicals  13 2.3.2  Carrier gas for thermal desorption  13 2.3.3  Diffusion denuders  13 2.3.4  Thermal desorption tubes  13 2.3.5  Hot gas spike apparatus  14 2.3.6  Outline of steps in method  14 2.3.7  Air sample collection  15 2.3.8  Thermal transfer from low-flow denuder into TD tube  15

Development of measurement and modeling techniques to quantify atmospheric deposition of persistent, bioaccumulative and toxic chemicals in the Great Lakes