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Manganite perovskites host emerging physical properties ofstrongly-correlated electrons with charge, spin, and lattice degrees offreedom. Using epitaxial lift-off technique, we report enhancement ofsaturation magnetization and ferromagnetic transition temperature of thefreestanding La2/3Sr1/3MnO3 membrane compared with the as-grown film on SrTiO3substrate involving lateral tensile strain. Structural analysis revealsshrinkage of unit-cell volume by tensile strain relaxation in the freestandingmembrane, which causes enhancement of the ferromagnetic interaction. The impactof the microscopic lattice deformation on the ferromagnetism of La2/3Sr1/3MnO3indicates a high potential of this material for flexible electronicsapplication with intriguing functionalities in strongly-correlated electronsystems.

Impact of epitaxial strain relaxation on ferromagnetism in a freestanding La2/3Sr1/3MnO3 membrane