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We successfully prepared two different classes of hypercrosslinked porous organic polymers (HPPs)-the tetraphenylethene (TPE) and (4-(5,6-Diphenyl-1H-Benzimidazol-2-yl)-triphenylamine (DPT) HPPs-through the Friedel-Crafts polymerization of tetraphenylethene and 4-(5,6-diphenyl-1H-benzimidazol-2-yl)-triphenylamine, respectively, with 1,4-bis(chloromethyl)benzene (Ph-2Cl) in the presence of anhydrous FeCl 3 as a catalyst. Our porous materials exhibited high BET surface areas (up to 1000 m 2 g -1 ) and good thermal stabilities. According to electrochemical and dyes adsorption applications, the as-prepared DPT-HPP exhibited a high specific capacitance of 110 F g -1 at a current density of 0.5 A g -1 , with an excellent cycling stability of over 2000 times at 10 A g -1 . In addition, DPT-HPP showed a high adsorption capacity up to 256.40 mg g -1 for the removal of RhB dye from water.

polymers

Multifunctional Hypercrosslinked Porous Organic Polymers Based on Tetraphenylethene and Triphenylamine Derivatives for High-Performance Dye Adsorption and Supercapacitor