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The interaction between single or a fixed number of photons with a single absorber is of fundamental interest in quantum technology. The harnessing of light matter interactions at the single particle limit has several potential applications ranging from quantum communication and quantum metrology to quantum imaging. In this perspective, a setup for heralded two-photon excited fluorescence at the single absorber level is proposed. The setup is based on a heralded two-photon source utilizing spontaneous parametric down-conversion, entanglement swapping and sum frequency generation for joint detection. This perspective aimed at triggering a discussion about the study of TPA and TPEF with only very few photons. The feasibility of the scheme is assessed by estimating the performance based on state-of-the-art technologies and losses, with the conclusion that the realization appears to be very challenging, but not completely impossible.

Is Heralded Two-Photon Excited Fluorescence with Single Absorbers Possible with Current Technology?