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Exploiting efficient electrocatalysts for hydrogen evolution reactions (HERs) is important for boosting the large-scale applications of hydrogen energy. Herein, MoP-RuP 2 encapsulated in N,P-codoped carbon (MoP-RuP 2 @NPC) with abundant interfaces were prepared via a facile avenue with the low-toxic melamine phosphate as the phosphorous resource. Moreover, the obtained electrocatalyst possessed a porous nanostructure, had abundant exposed active sites and improved the mass transport during the electrocatalytic process. Due to the above merits, the prepared MoP-RuP 2 @NPC delivered a greater electrocatalytic performance for HERs (50 mV@10 mA cm -2 ) relative to RuP 2 @NPC (120 mV) and MoP@NPC (195 mV) in 1 M KOH. Moreover, an ultralow potential of 1.6 V was required to deliver a current density of 10 mA cm -2 in the two-electrode configuration for overall water splitting. For practical applications, intermittent solar energy, wind energy and thermal energy were utilized to drive the electrolyzer to generate hydrogen gas. This work provides a novel and facile strategy for designing highly efficient and stable nanomaterials toward hydrogen production.

Facile Synthesis of MoP-RuP2 with Abundant Interfaces to Boost Hydrogen Evolution Reactions in Alkaline Media