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The incorporation of nonmetal group dopants into a graphitic carbon nitride (g-C 3 N 4 ) framework is fabricated by adding a small amount of hexamethylenetetramine during the thermal polymerization process. The material shows an excellent visible-light photocatalytic H 2 production performance that is eight times higher than bulk g-C 3 N 4 . This outstanding performance is ascribed to the introducing of N-doped carbon, which not only enhances the light absorption and favorsa narrower band gap, but also upshifts the conductionband (CB) potential, resulting in a better reduction ability of electrons. This discovery has potential significancefor the designing of high performance, economic, and environmental friendly photocatalyst for solar energy conversion.

Incorporation of Nonmetal Group Dopants into g-C3N4 Framework for Highly Improved Photocatalytic H2 Production