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This article demonstrates new observation of the high-resolution ro-vibrational bichromatic photoassociation spectra (BPAS) of Cs 2 in the 0u+ long-range state below the asymptotes 6S 1/2 + 6P 1/2 . By combining with a modulation spectroscopic technique, precise references of the frequency differences have been engineered through the BPAS, with which the rotational constants of low-lying vibrational levels of the Cs 2 0u+ long-range state have been accurately determined by fitting the frequency differences to the non-rigid-rotor model. The rotational constants for the newly observed seven ro-vibrational levels are summarized and disagreement for the level ῦ = 498 is clarified. The rotational constants of different vibrational levels demonstrate strong perturbations of the related energy structures. A simple analysis is performed and shows good agreement with experimental results.

molecules/molecules online/molecules annual

Bichromatic Photoassociation Spectroscopy for the Determination of Rotational Constants of Cs2 &#x0D; &#x0D; &#x0D; &#x0D; 0&#x0D; u&#x0D; +&#x0D; &#x0D; &#x0D; &#x0D; Long-Range State below the 6S1/2 + 6P1/2 Asymptote

Bichromatic Photoassociation Spectroscopy for the Determination of Rotational Constants of Cs2 0 u + Long-Range State below the 6S1/2 + 6P1/2 Asymptote