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the gamma-emitting radionuclide Technetium-99m ( 99m Tc) is still the workhorse of Single Photon Emission Computed Tomography (SPECT) as it is used worldwide for the diagnosis of a variety of phatological conditions. 99m Tc is obtained from 99 Mo/ 99m Tc generators as pertechnetate ion, which is the ubiquitous starting material for the preparation of 99m Tc radiopharmaceuticals. 99 Mo in such generators is currently produced in nuclear fission reactors as a by-product of 235 U fission. Here we investigated an alternative route for the production of 99 Mo by irradiating a natural metallic molybdenum powder using a 14-MeV accelerator-driven neutron source.

14 MeV Neutrons for 99Mo/99mTc Production: Experiments, Simulations and Perspectives