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Functionalized nanofluidics devices have recently emerged as a powerful platform for applications of energy conversion. Inspired by biological cells, we theoretically studied the effect of the interaction between the nanoparticle and the plate which formed the brush layer modified by functional zwitterionic polyelectrolyte (PE) on the bulk charge density of the nanoparticle brush layer, and the charge/discharge effect when the distance between the particle and the plate was changed. In this paper, The Poisson-Nernst-Planck equation system is used to build the theoretical model to study the interaction between the nanoparticle and the plate modified by the PE brush layer, considering brush layer charge regulation in the presence of multiple ionic species. The results show that the bulk charge density of the brush layer decreases with the decrease of the distance between the nanoparticle and the flat substrate when the interaction occurs between the nanoparticle and the plate. When the distance between the particle and the plate is about 2 nm, the charge density of the brush layer at the bottom of the particle is about 69% of that at the top, and the electric field energy density reaches the maximum value when the concentration of the background salt solution is 10 mm.

Charge Properties and Electric Field Energy Density of Functional Group-Modified Nanoparticle Interacting with a Flat Substrate