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In this study, the operation of donor/acceptor photovoltaic cells fabricated on homoepitaxially grown p -doped rubrene single-crystal substrates is demonstrated. The photocurrent density is dominated by the sheet conductivity (σ □ ) of the p -type single-crystal layer doped to 100 ppm with an iron chloride (Fe 2 Cl 6 ) acceptor. A 65 mm thick p- type rubrene single-crystal substrate is expected to be required for a photocurrent density of 20 mA·cm -2 . An entire bulk doping technique for rubrene single crystals is indispensable for the fabrication of practical organic single-crystal solar cells.

Donor/Acceptor Photovoltaic Cells Fabricated on p-Doped Organic Single-Crystal Substrates