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A series of carbazole-based polymers (PdCz, P(dCz2- co -dTC1), P(dCz2- co -dTC2), P(dCz1- co -dTC2), and PdTC) were deposited on indium tin oxide (ITO) conductive electrodes using electrochemical polymerization. The as-prepared P(dCz2- co -dTC2) displayed a high Δ T (57.0%) and multichromic behaviors ranging from yellowish green, greenish gray, gray to purplish gray in different redox states. Five organic electrochromic devices (ECDs) were built using dCz- and dTC-containing homopolymers and copolymers as anodic materials, and poly(3,4-(2,2-dimethylpropylenedioxy)thiophene) (PProdot-Me 2 ) as the cathodic material. The P(dCz2- co -dTC2)/PProdot-Me 2 ECD presented remarkable electrochromic behaviors from the bleached to colored states. Moreover, P(dCz2- co -dTC2)/PProdot-Me 2 ECD displayed a high optical contrast (Δ T , 45.8%), short switching time (ca. 0.3 s), high coloration efficiency (528.8 cm 2 C -1 ) at 580 nm, and high redox cycling stability.

Applications of Copolymers Consisting of 2,6-di(9H-carbazol-9-yl)pyridine and 3,6-di(2-thienyl)carbazole Units as Electrodes in Electrochromic Devices