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This work numerically determined high-energy photon shielding properties of self-healing poly(vinyl alcohol) (PVA) hydrogels containing lead-free, heavy-metal compounds, namely, bismuth oxide (Bi2O3), tungsten oxide (WO3), and barium sulfate (BaSO4), through XCOM software packages. In order to understand the dependencies of the shielding properties of the hydrogels on filler contents and photon energies, the filler contents added to the hydrogels were varied from 0–40 wt.% and the photon energies were varied from 0.001–5 MeV. The results, which were verified for their reliability and correctness with those obtained from PHITS (Particle and Heavy Ion Transport code System), indicated that overall shielding performances, which included the mass attenuation coefficients (µm), the linear attenuation coefficient (µ), the half-value layer (HVL), and the lead equivalence (Pbeq), of the hydrogels improved with increasing filler contents but generally decreased with increasing photon energies. Among the three compounds investigated in this work, Bi2O3/PVA hydrogels exhibited the highest photon attenuation capabilities, determined at the same filler content and photon energy, mainly due to its highest atomic number of Bi and the highest density of Bi2O3 in comparison with other elements and compounds. Furthermore, due to possible reduction in self-healing and mechanical properties of the hydrogels with excessive filler contents, the least content of fillers providing a 10-mm sample with the required Pbeq value of 0.5 mmPb was investigated. The determination revealed that only the hydrogel containing at least 36 wt.% of Bi2O3 exhibited the Pbeq values greater than 0.5 mmPb for all photon energies of 0.05, 0.08, and 0.1 MeV (common X-ray energies in general nuclear facilities). The overall outcomes of the work promisingly implied the potential of PVA hydrogels to be used as novel and potent X-ray and gamma shielding materials with the additional self-healing and nonlead properties.

High-Energy Photon Attenuation Properties of Lead-Free and Self-Healing Poly (Vinyl Alcohol) (PVA) Hydrogels: Numerical Determination and Simulation