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The proper hydrogenation of Hyper-coal (HPC) using 1,2,3,4-tetrahydroquinoline (THQ) was able to decrease the oxygen content and adjust the molecular structure of HPC for preparing the spinnable pitch with high softening point (SP). The spinnable pitch prepared from the THQ-soluble (QS) fraction of HPC as a precursor consisted of more naphthenic carbon groups than that prepared from the 1-methylnaphthalene (1-MN) soluble (MNS) fraction of HPC. The HPC-QS derived spinnable pitch showed excellent spinning performance even though the SP of 260 °C, and the tensile strength of the resultant carbon fiber was increased to 1350 MPa with a diameter around 8 µm under the only carbonization temperature of at 800 °C for 5 min.

Improving Spinnability of Hyper-Coal Derived Spinnable Pitch through the Hydrogenation with 1,2,3,4-Tetrahydroquinoline