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With the intensification of global warming and economic development in China, the near-surface ozone (O3) concentration has been increasing recently, especially in the Beijing-Tianjin-Hebei (BTH) region, which is the political and economic center of China. However, O3 has been measured in real time only over the past few years, and the observational records are discontinuous. Therefore, we propose a new method (WRFC-XGB) to establish a near-surface O3 concentration dataset in the BTH region by integrating the Weather Research and Forecasting with Chemistry (WRF-Chem) model with the extreme gradient boosting (XGBoost) algorithm. Based on this method, the 8-h maximum daily average (MDA8) O3 concentrations are obtained with full spatiotemporal coverage at a spatial resolution of 0.1° × 0.1° across the BTH region in 2018. Two evaluation methods, sample- and station-based 10-fold cross-validation (10-CV), are used to assess our method. The sample-based (station-based) 10-CV evaluation results indicate that WRFC-XGB can achieve excellent accuracy with a high coefficient of determination (R2) of 0.95 (0.91), low root mean square error (RMSE) of 13.50 (17.70) µg m−3, and mean absolute error (MAE) of 9.60 (12.89) µg m−3. In addition, superb spatiotemporal consistencies are confirmed for this model, including the estimation of high O3 concentrations, and our WRFC-XGB model outperforms traditional models and previous studies in data mining. In addition, the proposed model can be applied to estimate the O3 concentration when it has not been measured. Furthermore, the spatial distribution analysis of the MDA8 O3 in 2018 reveals that O3 pollution in the BTH region exhibits significant seasonality. Heavy O3 pollution episodes mainly occur in summer, and the high O3 loading is distributed mainly in the southern BTH areas, which will pose challenges to atmospheric environmental governance for local governments.

atmosphere

Estimation of the Near-Surface Ozone Concentration with Full Spatiotemporal Coverage across the Beijing-Tianjin-Hebei Region Based on Extreme Gradient Boosting Combined with a WRF-Chem Model