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Uncertainty is a common feature in first-principles models that are widely used in various engineering problems. Uncertainty quantification (UQ) has become an essential procedure to improve the accuracy and reliability of model predictions. Polynomial chaos expansion (PCE) has been used as an efficient approach for UQ by approximating uncertainty with orthogonal polynomial basis functions of standard distributions (e.g., normal) chosen from the Askey scheme. However, uncertainty in practice may not be represented well by standard distributions. In this case, the convergence rate and accuracy of the PCE-based UQ cannot be guaranteed. Further, when models involve non-polynomial forms, the PCE-based UQ can be computationally impractical in the presence of many parametric uncertainties. To address these issues, the Gram–Schmidt (GS) orthogonalization and generalized dimension reduction method (gDRM) are integrated with the PCE in this work to deal with many parametric uncertainties that follow arbitrary distributions. The performance of the proposed method is demonstrated with three benchmark cases including two chemical engineering problems in terms of UQ accuracy and computational efficiency by comparison with available algorithms (e.g., non-intrusive PCE).

An Efficient Polynomial Chaos Expansion Method for Uncertainty Quantification in Dynamic Systems