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Organic-inorganic hybrid methylammonium lead halide perovskite MAPbX3 (where MA = CH 3 NH 3 , and  X  = Cl, Br, I) single crystals are potential semiconductors for photo-detection due to their excellent optoelectronic performance. In particular, MAPbCl 3  single crystal is a wide-band-gap (2.9 eV) semiconductor which is suitable for ultraviolet (UV) detection. In this work, n − -n +  photo-diodes are fabricated through solution-processed epitaxial growth, growing Bi-doped MAPbCl 3  epitaxial layer on MAPbCl 3  single crystal substrate. The epitaxial layer effectively improves the interface between n − -type and n + -type layers and leads to low dark current. This work provides useful information for UV detection based on perovskites.

Photo-Diodes Based on CH3NH3PbCl3 Perovskite Single Crystals by Epitaxial Growth for Ultraviolet Photo-Detection