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HIGHLIGHTS • We observed Autler-Townes splitting of single peak into two and three peaks in two-level, and three-level systems, respectively. • We reported primary and secondary Autler-Townes splitting are caused by double cascaded dressing in time domain. • WeobservedAutler-Townessplittingofmulti-orderfluorescenceintimedomainismore obvious than that of in spectral domain. For first time, we study primary and secondary Autler-Townes (AT) splitting of multi-order fluorescence (FL) in time domain. The AT-splitting of multi-order FL signals are controlled by changing power, detuning, and polarization of single and double dressing in a heteronuclear-like molecule system of Pr C3 :YSO. The primary and secondary AT-splitting are caused by double cascaded dressing in time domain. The AT-splitting of multi-order FL in time domain is more sensitive than that of in spectral domain. Such results have potential applications in quantum communication and optical information processing on photonic chip.

Lifetime Autler-Townes Splitting of Dressed Multi-Order Fluorescence in Pr3+:YSO