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The nonlinear magneto-optical Kerr effect on a Fe(110) surface and its dependence on the oxygen exposure is investigated at a wavelength of the incident light of 790 nm for different geometries. Especially for the transverse Kerr geometry a large intensity change upon reversal of the magnetization direction by a factor more than 4 is observed which can be increased to 80 by oxygen exposure. The magnetization induced part of the nonlinear susceptibility tensor is comparable in size to the nonmagnetic part.

OBSERVATION OF VERY LARGE MAGNETIC CONTRAST IN THE SECOND HARMONIC GENERATION FROM Fe(110)