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It is well-known that strength and stiffness are commonly inversely related with toughness and ductility for organic filler filled elastomer nanocomposites. These performances are governed by the dispersion of organic fillers and interface of elastomer nanocomposites. Herein, the designed physical and chemical hybrid-network based on tannic acid (TA) as interface regulator and cross-link agent can endow graphene/elastomer nanocomposites with reinforcement as well as toughness simultaneously. The results indicate the formation of a strong and stable network structure composed of elastomer chains and graphene, contrary to traditional graphene/elastomer nanocomposites. The present composites with a physical and chemical hybrid-network effectively improve the load transfer and show excellent mechanical properties.

High-Performance Natural Rubber/Graphene Composites from a Uniquely Designed Physical and Chemical Hybrid-Network