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Light interacting with nanostructured metals excites collective charge density ‰uctuations known as surface plasmons. By combining interferometric time-resolved two-photon photoemission and photoemission electron microscopy, we demonstrate imaging of surface plasmon dynamics with 60 nm spatial resolution and 0.33 fs frame interval. 10 fs phase-correlated pump-probe light pulses at 400 nm couple to localized and/or propagating surface plasmon modes in structured silver ˆlms that mediate nonlinear tow-photon photoemission from the samples.

Femtosecond Time-resolved Photoemission Electron Microscope Studies of Surface Plasmon Dynamics