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77 INTRODUCTION 78 DEVELOPMENT OF THE TWO-DIMENSIONAL GRAIN MODEL 79 Method of Solution 82 RESULTS AND DISCUSSION 84 Evaluation of the Thiele-Type Modulus 86 Equivalent Spherical Radius Approximation 86 Infinite Cylinder Approximation 86 Infinite Slab Approximation 92 Experimental Determination of Rate Constants 92 CONCLUSIONS 98 NOTATION 99 REFERENCES 101 PART III, A MORE STABLE NUMERICAL SOLUTION TECHNIQUE FOR THE GRAIN MODEL IN SOLID-GAS REACTIONS 102 INTRODUCTION 103 GRAIN MODEL 104 ANALYSIS OF SOLUTION METHOD 105 SUMMARY AND CONCLUSIONS 111 NOTATION 112 REFERENCES 113

Modeling of solid-gas reactions with application to the chlorination of lime