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The proposed time-resolved spe trometry is of high temporal resolution within the femtose ond s ale. Re ently, performing of real-time studies of mole ular dynami s is of great interest. The photoele tron spe trometry exhibits high sensitivity, sin e photoionization is an indu ed pro ess and the ele trons an be olle ted eÆ iently by an ele tromagneti eld. Su h method is applied to ultrafast dephasing pro ess in mole ular pyrazine. The photoele tron imaging allows measurements of speed and angular distributions with unit olle tion eÆ ien y of ele trons. We should note that the photoele tron imaging probes short range and short time dynami s involving the ele troni relaxation. The method is hara terized by photoionization of NO and further applied to ultrafast dephasing in pyrazine. The ombination of time-resolved photoele tron and photoion imaging will allow us to observe photo-indu ed dynami s of mole ules and lusters from time t = 0 to 1 with a single apparatus. The experimental results are ompared with the theoreti al analysis of strong impa t onto the multi-ele tron systems.

Time-resolved photoelectron spectrometry of a dephasing process in pyrazine