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In this paper, using aniline, lauryl alcohol and nonanoic acid as the structural controlling reagents, hierarchical mesoporous TiO2 microspheres composed of connected nanoparticles are synthesized via a coupled sol-gel and solvothermal process. The dye sensitized solar cells (DSSCs) with the mesoporous TiO2 microspheres as photoanodes demonstrate light to electricity conversion efficiency ranges from 3.9 to 6.5 %, dramatically higher than that made of P25 (3.26 %).

The Structures and Properties of Hierarchical Mesoporous TiO2 Microspheres in Dye sensitized Solar Cells Controlled by Different Reagents