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Solvent effect is investigated on β-phophorylated nitroxides carrying electron widthdrawing groups exhibiting various steric hindrances. Solvent effect on nitrogen and phosphorus hyperfine coupling constants highlights the entanglement of polar and steric effects on the changes in hyperfine coupling constants.

Cybotactic Effect on Nitrogen and Phosphorus Hyperfine Coupling Constants in β-Phosphorylated Nitroxides.