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Chapter 1 reports a highly sensitive and selective array-based sensing strategy for classifying isomeric and analogous analytes based on their differential interactions with three supramolecular cyclodextrin-fluorophore sensors. Each analyte-sensor interaction results in a distinct fluorescence modulation response, and these variable responses are then statistically classified via linear discriminant analyses (LDA) into clusters of maximum separation. Three classes of isomeric analytes (aromatic alcohols, aliphatic alcohols, and hexanes) and two classes of analogous analytes (analogues of dichlorodiphenyltrichloroethane (DDT) and congeners of polychlorinated biphenyls (PCBs)) have been successfully classified with 100% accuracy. High sensitivity of this sensor is demonstrated as well, with limits of detection approaching or surpassing known levels of concern, and preliminary efforts at successfully classifying binary analyte mixtures using this sensor system are also

Toxicant Isomers Characteized Using Fluorescence Emission of Coumarin Attached to Beta-Cyclodextrin