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Mould fluxes play a very important role in the continuous casting of steel. The mould flux infiltrates into the steel shell and the mould, and exists layer by layer, typically in the form of a glassy phase next to the mould, a partially crystallised phase and a liquid phase next to the shell. Mould fluxes are required to have several functions including (i) lubrication between the steel shell and the mould and (ii) heat extraction rate control from the molten steel.1) The former function is primarily related to viscosity2,3) and the latter function to thermal conductivity4,5) and optical properties.6–10) Thus, the physical properties of mould fluxes have been investigated by many workers for a long time.11) In addition to the physical properties, in practice, the types of mould flux are selected from many perspectives including the mould geometry and the steel grade. For the mould Crystallisation of Silicate Glasses and Melts with Chemical Compositions in Primary Phase Region of Gehlenite