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Solidification is a key step in the processing of metal materials. The rheological behavior of metal melts during solidification can provide remarkable insight into the process operations and the product quality of the resulting alloys. In the steelmaking process, the formation of product defects, such as porosity, element segregation and shrinkage, is closely related to the viscosity of the Fe–C melts during solidification because the viscosity of the melt controls the fluidity and the rate of transport of the liquid metal.1) Therefore, determining the apparent viscosities of Fe–C melts during solidification is of great significance when guiding the production of these materials. There have been many previous studies investigating the viscosity of pure liquid metals as well as non-ferrous and low melting point metals in the semi-solid state, providing a wide library of experimental data in the literature.2–5) However, the data on the apparent viscosity of Fe–C melts during solidification is extremely limited due to the experimental difficulties such as the poor availability of rheological instruments for use at high temperatures and a measurement spindle that does not react with the molten Fe–C alloy. Shibutani et al.6) measured the apparent viscosity of Fe–C (3 and 4%C) and Fe–Cr–Ni–C alloys in state where liquid and solid phases coexisted using rotating coaxial Measurement and Characterization of the Apparent Viscosity of Fe–C Melts during Solidification