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The Block and randam co-oligomers were synthesized by radical re- or co-telomerization of methacrylate monomer with fluoroalkyl group and styrene in carbon tetrabromide as a telogen. Using both co-oligomers, FKM/EPDM blends can be easily obtained and physical properties of vulcanized FKM/EPDM blends are improved compared with vulcanized control blend. From these results, it was recognized that co-oligomers show the action of compatibilizer and co-vulcanizing agent. The effect of surface modification of block co-oligomer on EPDM vulcanizates was remarkable, but the difference between block and randam co-oligomer on physical properties of rubber blends was poorly characterized.

Improvement in Properties of Rubber with Co-oligomer Containing Fluorine Atom, Part 2.